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Guang-Zhong Xie, Ting Kang, Yong Zhou, Tao Xie, Hui-Ling Tai, Ya-Dong Jiang. QCM Sensors Based on PEI Films for CO2 Detection[J]. Journal of Electronic Science and Technology, 2015, 13(2): 181-187. DOI: 10.3969/j.issn.1674-862X.2015.02.017
Citation: Guang-Zhong Xie, Ting Kang, Yong Zhou, Tao Xie, Hui-Ling Tai, Ya-Dong Jiang. QCM Sensors Based on PEI Films for CO2 Detection[J]. Journal of Electronic Science and Technology, 2015, 13(2): 181-187. DOI: 10.3969/j.issn.1674-862X.2015.02.017
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QCM Sensors Based on PEI Films for CO2 Detection

doi: 10.3969/j.issn.1674-862X.2015.02.017

  • School of Optoelectronic Information,University of Electronic Science and Technology of China,Chengdu 610054,China

Funds: 

This work was supported by the National Natural Science Foundation of China under Grant No. 61176006 and No. 61006036, and the Specialized Research Fund for the Doctoral Program of Higher Education under Grant No. 20120185110012.

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  • Author Bio:

    Guang-Zhong Xie research interests are sensitive materials and sensors, gzxie@uestc.edu.cn;
    Ting Kang, xiaobu0401@126.com;
    Yong Zhou, zhyfly68@126.com;
    Tao Xie, Xietaohlj@163.com;
    Hui-Ling Tai, taitai1980@uestc.edu.cn;
    Ya-Dong Jiang, jiangyd@uestc.edu.cn

    Guang-Zhong Xie research interests are sensitive materials and sensors, gzxie@uestc.edu.cn;
    Ting Kang, xiaobu0401@126.com;
    Yong Zhou, zhyfly68@126.com;
    Tao Xie, Xietaohlj@163.com;
    Hui-Ling Tai, taitai1980@uestc.edu.cn;
    Ya-Dong Jiang, jiangyd@uestc.edu.cn

    Guang-Zhong Xie research interests are sensitive materials and sensors, gzxie@uestc.edu.cn;
    Ting Kang, xiaobu0401@126.com;
    Yong Zhou, zhyfly68@126.com;
    Tao Xie, Xietaohlj@163.com;
    Hui-Ling Tai, taitai1980@uestc.edu.cn;
    Ya-Dong Jiang, jiangyd@uestc.edu.cn

    Guang-Zhong Xie research interests are sensitive materials and sensors, gzxie@uestc.edu.cn;
    Ting Kang, xiaobu0401@126.com;
    Yong Zhou, zhyfly68@126.com;
    Tao Xie, Xietaohlj@163.com;
    Hui-Ling Tai, taitai1980@uestc.edu.cn;
    Ya-Dong Jiang, jiangyd@uestc.edu.cn

    Guang-Zhong Xie research interests are sensitive materials and sensors, gzxie@uestc.edu.cn;
    Ting Kang, xiaobu0401@126.com;
    Yong Zhou, zhyfly68@126.com;
    Tao Xie, Xietaohlj@163.com;
    Hui-Ling Tai, taitai1980@uestc.edu.cn;
    Ya-Dong Jiang, jiangyd@uestc.edu.cn

    Guang-Zhong Xie research interests are sensitive materials and sensors, gzxie@uestc.edu.cn;
    Ting Kang, xiaobu0401@126.com;
    Yong Zhou, zhyfly68@126.com;
    Tao Xie, Xietaohlj@163.com;
    Hui-Ling Tai, taitai1980@uestc.edu.cn;
    Ya-Dong Jiang, jiangyd@uestc.edu.cn

  • Authors’ information: Guang-Zhong Xie
  • Received Date: 2014-08-31
  • Rev Recd Date: 2014-11-03
  • Publish Date: 2015-06-24
    Abstract
  • In this paper, quartz crystal microbalance (QCM) gas sensors coated with polyehtyleneimine (PEI) was utilized for carbon dioxide (CO2) detection. The sensing mechanism is based on the availability of reversible acid-base reactions between CO2 molecules and PEI at room temperature. The experimental results revealed that the PEI/starch sensor exhibited much higher sensitivity than that of pure PEI, and showed approximate linearity over a concentration region ranging from 500 ppm to 8000 ppm. The influence of humidity had also been investigated. Furthermore, the response and recovery time deceased as the operation temperatures increased. Finally, sensitivity loss after conservation for several days and reversibility of the sensors had been discussed.
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    1. Na Songkhla, S.. Quartz crystal microbalance sensors. Digital Technologies in Olfaction: Fundamentals to Applications, 2025. DOI:10.1016/B978-0-443-15721-9.00004-X
    2. Siefker, Z.A., Hodul, J.N., Flores-Hansen, C. et al. Sorption Kinetics of Poly(ethyleneimine)-Poly(ethylene Oxide) Blends and the Implication for Low-Cost, Small-Scale CO2Sensors. ACS Applied Polymer Materials, 2022, 4(6): 4389-4397. DOI:10.1021/acsapm.2c00361
    3. Siefker, Z.A., Hodul, J.N., Zhao, X. et al. Manipulating polymer composition to create low-cost, high-fidelity sensors for indoor CO2 monitoring. Scientific Reports, 2021, 11(1): 13237. DOI:10.1038/s41598-021-92181-4
    4. Ersöz, B., Schmitt, K., Wöllenstein, J. Electrolyte-gated transistor for CO2 gas detection at room temperature. Sensors and Actuators, B: Chemical, 2020. DOI:10.1016/j.snb.2020.128201
    5. Su, Y., Xie, G., Wang, S. et al. Novel high-performance self-powered humidity detection enabled by triboelectric effect. Sensors and Actuators, B: Chemical, 2017. DOI:10.1016/j.snb.2017.04.039
    6. Ma, X.F., Xie, G.Z., Su, Y.J. et al. Polyvinylpyrrolidone/graphene oxide thin films coated on quartz crystal microbalance electrode for NH3 detection at room temperature. Science China Technological Sciences, 2016, 59(9): 1377-1382. DOI:10.1007/s11431-016-0281-7

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